Home >  About ISSP >  Publications > Activity Report 2024 > Magnon Thermal Hall Effect on the Antiferromagnetic Skyrmion Lattice

Magnon Thermal Hall Effect on the Antiferromagnetic Skyrmion Lattice

Yamashita Group

Recently, transport phenomena involving quantum quasiparticles other than electrons have attracted significant interest in both fundamental and applied sciences. A prominent example is the magnon, a magnetic quasiparticle that propagates through magnetic insulators and carries heat and spin without electric charge. Due to their charge neutrality, magnons do not experience the Lorentz force and typically do not exhibit transverse transport under an external magnetic field, i.e., the thermal Hall effect in conventional insulators. However, when certain conditions are satisfied in the spin interactions or magnetic structure of a material, an emergent gauge field—a fictitious magnetic field—can arise and induce a magnon thermal Hall effect. This phenomenon has been interpreted in terms of emergent U(1)\mathrm{U}(1) gauge fields, which can give rise to a nonzero thermal Hall conduction in materials with corner-sharing lattice geometries such as kagome and pyrochlore lattices. In contrast, for edge-sharing lattices such as square or triangular lattices, a so-called “no-go theorem” predicts the strict cancellation of the Hall conduction due to the commutative nature of the U(1)\mathrm{U}(1) gauge field. As a result, magnon thermal Hall effects in edge-sharing lattices have long been considered unlikely, with rare exceptions such as our previous work [1] done in the ferromagnetic skyrmion lattice in GaV4Se8.

yamashita-fig1.jpg
Fig. 1. (a) Diamond lattice formed by Mn2+ ions in MnSc2S4. The two (111) planes marked in blue include Mn2+ ions belonging to different sublattice of the bipartite diamond structure. (b) Schematic figure of the AFM-SkL state in MnSc2S4 viewed along [111] direction.

In this study [2], we have demonstrated that the spinel compound MnSc2S4, in which Mn atoms form a diamond lattice (Fig. 1(a)), exhibits a magnon-induced thermal Hall effect. This material undergoes antiferromagnetic ordering below approximately 2.3 K and, under magnetic fields of about 4–6 T, enters a novel magnetic phase known as an antiferromagnetic skyrmion lattice (AFM-SkL) composed of three interpenetrating sublattices (Fig. 1(b)). Each sublattice hosts a ferromagnetic skyrmion lattice, and collectively they form a 120 antiferromagnetic configuration. Thermal transport measurements reveal a sharp increase in the thermal Hall conductivity by magnons within the AFM-SkL phase region, ollowed by a gradual decrease while retaining a positive value above 8 T (Fig. 2).

yamashita-fig2.jpg
Fig. 2. Field dependence of thermal Hall conductivity divided by temperature κxy/T in the magnetically ordered phases. The shaded area represents the AFM-SkL phase.

This experimental result goes beyond conventional understanding based on U(1)\mathrm{U}(1) gauge fields, which cannot account for a finite Hall conductivity in edge-sharing lattices. Theoretical analysis based on the spin texture of the AFM-SkL reveals that an emergent SU(3)\mathrm{SU}(3) gauge field arises from the system. The three U(1)\mathrm{U}(1) gauge fields associated with each sublattice couple via off-diagonal spin interactions and form a non-Abelian SU(3)\mathrm{SU}(3) gauge structure. The non-commutativity of SU(3)\mathrm{SU}(3) enables a net emergent magnetic flux that does not cancel out, allowing a finite magnon thermal Hall effect even in edge-sharing lattices. This work presents the first experimental signature of an emergent SU(3)\mathrm{SU}(3) gauge field in a solid-state system and highlights how the topological nature of magnetic order can fundamentally alter magnon transport, paving the way for new functional properties in quantum magnetic materials.


References
  • [1] M. Akazawa et al., Phys. Rev. Research 4, 043085 (2022).
  • [2] H. Takeda et al., Nature Commun. 15, 566 (2024).
Authors
  • H. Takeda, M. Kawanoa, K. Tamura, M. Akazawa, J. Yan, T. Wakib, H. Nakamurab, K. Satoc, Y. Narumic, M. Hagiwarac, M. Yamashita, and C. Hottad
  • aDepartment of Physics, Technical University of Munich
  • bDepartment of Materials Science and Engineering, Kyoto University
  • cCenter for Advanced High Magnetic Field Science, Graduate School of Science, Osaka University
  • dDepartment of Basic Science, University of Tokyo