Gapless Magnon-Driven Anomalous Hall Conductivity in the Collinear Kagome Antiferromagnet YbFe6Ge6
PI of Joint-use project: P. Dai
Host lab: Masuda Group and Kindo Group
Host lab: Masuda Group and Kindo Group
YbFe6Ge6 is a kagome-lattice intermetallic whose Fe3+ moments order antiferromagnetically below 500 K. Neutron diffraction shows an A-type structure with spins along the axis above the spin-reorientation temperature 63 K; on cooling the moments rotate into the kagome plane while the propagation vector remains , preserving inversion–time-reversal symmetry and eliminating static scalar chirality [1]. Magnetotransport reveals that this reorientation generates an anomalous Hall conductivity 30 Ω-1 cm-1 at 10 K for in-plane fields, whereas no signal appears for out-of-plane fields or , confirming its anisotropy dependence rather than any coupling to net magnetization [1].
Low-energy spin dynamics were resolved by inelastic neutron scattering. As shown in Fig. 1(a) [1], magnetic intensity at in the spin-reoriented phase is continuous up to 0.6 meV, defining a gapless magnon branch above the 0.14 meV resolution. The temperature evolution of intensities at 0.55 meV and 2.55 meV, plotted in Fig. 1(b) [1], demonstrates that the gap remains closed throughout the easy-plane phase and reopens abruptly at TSR, growing to 1.34 meV by 80 K. The concomitant loss of , reproduced in Fig. 1(c) [1], shows a one-to-one correspondence between gapless magnons and Hall response: whenever the sub-meV continuum vanishes, the transverse conductivity collapses. A 7 T field also quenches ; its Zeeman energy for the 1.5 Fe moment is 0.6 meV, matching the upper edge of the gapless band and reinforcing the causal link.
Because the combined space inversion and time-reversal (IT) symmetry eliminates equilibrium Berry curvature and the magnetization never exceeds 0.3 /Fe even at 50 T, conventional intrinsic or skew-scattering mechanisms are excluded. Instead, propagating magnons transiently cant neighboring Fe moments; coupling to partially polarized Yb3+ spins biases the distribution of local scalar chiralities, creating a net dynamic Berry phase that deflects itinerant electrons. When the magnon gap opens thermally or via Zeeman splitting these fluctuations are suppressed and the Hall signal disappears [2]. Comparable fluctuation-driven Hall effects in kagome ferromagnets Mn6Sn6 [3] and in Fe3Sn2 [4] require non-collinear ground states, yet YbFe6Ge6 shows that collinear antiferromagnets can host the same physics provided that low-energy magnons are gapless. The absence of any Hall signal in FeSn, whose gap stays near 2 meV at all temperatures, underscores the necessity of near-zero-energy modes [5]. Only the quasi-acoustic branch softens across TSR; higher-energy magnons up to 40 meV remain unchanged, indicating that anisotropy rather than exchange drives the soft mode. Integrating the inelastic intensity yields a fluctuating Fe moment of ≈ 1.5 , consistent with diffraction and validating the local-moment picture. These results demonstrate that centrosymmetric, magnetically compensated antiferromagnets can exhibit field-controllable topological transport when anisotropy collapses the magnon gap to zero, extending antiferromagnetic spintronics beyond systems with static chirality and suggesting that engineered soft-mode transitions could enable chirality-mediated charge–spin conversion at terahertz frequencies [6].
References
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- [2] W. Wang et al., Nat. Mater. 18, 1054 (2019).
- [3] N. Ghimire et al., Sci. Adv. 6, eabe2680 (2020).
- [4] M. Kang et al., Nat. Mater. 19, 163 (2020).
- [5] S.-H. Do et al., Phys. Rev. B 105, L180403 (2022).
- [6] Y. Fujishiro et al., Nat. Commun. 12, 317 (2021).